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- W2020321024 abstract "Abstract Evidence has appeared in the literature that ignition-extinction phenomena in heterogeneously catalyzed reactions can be induced by pure kinetic effects. This paper presents an elegant and simple analytical reasoning based upon elementary properties of polynomials to derive explicit necessary and sufficient conditions for this behaviour for various reaction mechanisms, including Langmuir as well as non-Langmuir-type of adsorption. It is inspired on geometric arguments on the steady state equation, involving tangent adsorption and surface reaction rate curves as a function of surface coverage, which represent the limiting cases of rate multiplicity. The approach is particularly attractive for Langmuir-type adsorption as the adsorption rate equations are linear in this case. The technique is also applicable with the same ease in most situations of nonlinear adsorption characteristics and is to be preferred over a number of more intricate alternatives, because of its simplicity and its ability of defining explicit maximal bounds on the fundamental parameters." @default.
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- W2020321024 modified "2023-09-27" @default.
- W2020321024 title "Kinetically induced unstable behaviour in heterogeneously catalyzed reactions" @default.
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- W2020321024 doi "https://doi.org/10.1016/0009-2509(85)85086-7" @default.
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