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- W2020431311 abstract "The lowest lying vibrational bands of the gas-phase spectra of cyanogen, NCCN, and four of its isotopomers, 15NCCN, N13CCN, 15NCC15N, and N13C13CN, were recorded with a Fourier transform interferometer. The resolution was limited by the maximum optical path difference (MOPD) attainable with the interferometer to FWHM=0.0012cm−1. Rovibrational transitions of the ν5 (≈230cm−1) and also the ν2–ν5 (≈610cm−1) band systems were assigned for all five isotopomers. The use of an effective Hamiltonian for linear molecules to fit the data yielded precise spectroscopic vibrational and rotational constants for the vibrational states (v1v2v3v4v5) or (v4v5)=(00), (01), (02), (03), and (01000). These data include the first rotationally resolved transitions involving (01000). Complete substitution (rs) structures of cyanogen, based on both single and double isotopic substitution of the parent species, were calculated. The derived structure is rCC=138.48(17) pm and rCN=115.66(13) pm. The two rs structures coincide within the errors due to remaining contributions of zero-point vibrations." @default.
- W2020431311 created "2016-06-24" @default.
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- W2020431311 date "2003-04-01" @default.
- W2020431311 modified "2023-10-11" @default.
- W2020431311 title "Substitution structure of cyanogen, NCCN, from high-resolution far infrared spectra" @default.
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- W2020431311 doi "https://doi.org/10.1016/s0022-2852(02)00092-9" @default.
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