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- W2020471232 abstract "Designing and controlling the anode–electrolyte interfacial chemistry of a micron Sn-Ni/graphite composite battery anode led to the formation of a stable solid electrolyte interphase (SEI) layer. We utilized fluoroethylene carbonate (FEC)-based electrolyte that is more interfacially compatible than an EC-based electrolyte, trimethyl phosphite electrolyte additive that reduces the attack of LiPF6-derived acidic species in the electrolyte, and the addition of a low fraction of SnF2 to anode for capturing the F anions of HF present in the electrolyte. Mechanistic surface chemistry studies using ATR FTIR and X-ray photoelectron spectroscopy revealed that the SnF2 transforms to SnF4 by capturing F anions, while FEC and phosphite provide a surface protective and robust SEI. The interfacially controlled composite anode with a tuned content of graphite exhibits good cycling stability (90% retention at the 50th cycle) with high discharge capacity of ∼800 mAhg−1 of tin, in contrast to a rapid capacity fade in the conventional electrolyte." @default.
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- W2020471232 date "2014-01-01" @default.
- W2020471232 modified "2023-10-16" @default.
- W2020471232 title "Interfacial Chemistry Control for Performance Enhancement of Micron Tin-Nickel/Graphite Battery Anode" @default.
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- W2020471232 doi "https://doi.org/10.1149/2.0661412jes" @default.
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