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• W2020512096 abstract "Gas-phase line shapes and band contours are calculated for microwave spectra involving fine structure levels due to electron spin and/or orbital angular momentum, or vibrational angular momentum. We use the impact approximation, and a semiclassical treatment of the molecular rotation. The line shapes are expressed in terms of a set of cross sections which depend on the transfer of angular momentum by collisions. Different results are found, depending on whether the spin and rotation are coupled together strongly [Case (a)] or weakly [Case (b)]. Good agreement is obtained with microwave measurements on NO [Case (a)] and O2 [Case (b)]. The results may be applied to study the angle-dependent shape of intermolecular forces." @default.
• W2020512096 created "2016-06-24" @default.
• W2020512096 creator A5005030015 @default.
• W2020512096 date "1967-01-15" @default.
• W2020512096 modified "2023-09-23" @default.
• W2020512096 title "On the Pressure Broadening of Molecular Multiplet Spectra" @default.
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• W2020512096 doi "https://doi.org/10.1063/1.1840686" @default.
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