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- W2020596486 abstract "Carboxylate assistance was key to success for highly efficient ruthenium-catalyzed direct ortho-arylations of tetrazolyl-substituted arenes with aryl halides and triflates in the absence of phosphine ligands. Thus, ruthenium(II) biscarboxylates allowed for C–H bond functionalizations with excellent chemo- and site-selectivities, which set the stage for an atom- and step-economical access to key angiotensin-II-receptor blockers. Mechanistic studies revealed the C–H bond metalation to be reversible, and were suggestive of a rate-determining reductive elimination." @default.
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- W2020596486 date "2013-06-01" @default.
- W2020596486 modified "2023-09-24" @default.
- W2020596486 title "Carboxylate-assisted ruthenium(II)-catalyzed C–H arylations of 5-aryl tetrazoles: step-economical access to Valsartan" @default.
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- W2020596486 doi "https://doi.org/10.1016/j.tet.2013.01.006" @default.
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