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- W2020693864 abstract "A method is proposed, allowing to apply the many-body model of universal dielectric response, expressed in time domain as j ≈[(αt)n + (αt)1+m]−1, to solve the equations of thermally stimulated discharge (TSD). An approximate solution is obtained for a general case and an exact one for the condition m = 1 − n. The model many-body TDS curves show typical features inherent to experimental spectra (broad maxima, “initial rise” of the activation energy depending on the width parameter m, etc.), but contrary to experimental results the position and shape of the model TSD peaks do not depend on polarization and depolarization conditions. It is concluded that the many-body model, at least in its present formulation is not suitable to interpret the dielectric properties of polymers, especially in non-isothermal regime.Es wird eine Methode vorgeschlagen, die sich auf das Vielteilchen-Modell der universalen dielektrischen Response anwenden last, ausgedruckt im Zeitbereich durch j ≈ [(αt)n + (αt)1+m]−1, um die Gleichungen der thermisch stimulierten Entladung (TSD) zu losen. Eine Naherungslosung fur einen allgemeinen Fall und eine exakte Losung fur die Bedingung m = 1 − n wird erhalten. Die Modellkurven der Vielteilchen-TSD zeigen typisches Verhalten der experimentellen Spektren (breite Maxima, “Anfangsanstiegs”-Aktivierungsenergie in Abhangigkeit vom Breitenparameter m, usw.), jedoch im Gegensatz zu den experimentellen Ergebnissen hangt die Lage und Form der Modell-TSD-Maxima nicht von den Polarisations- und Depolarisationsbedingungen ab. Es wird geschlossen, das das Vielteilchenmodell, wenigstens in seiner gegenwartigen Formulierung, nicht geeignet ist fur die Interpretation der dielektrischen Eigenschaften von Polymeren, insbesondere im nicht-isothermen Bereich." @default.
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- W2020693864 title "On the application of the many-body model of universal dielectric response to thermally stimulated depolarization" @default.
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- W2020693864 doi "https://doi.org/10.1002/pssa.2210580209" @default.
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