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- W2020737476 abstract "The merits of UV-visible diffuse reflectance spectroscopy for the study of surface phenomena on microcrystalline MgO, CaO and SrO are described and illustrated. It is shown that surface states ascribable to anions in 5-, 4- and 3-coordination can be observed and their respective interactions with adsorbed gases investigated. The behaviour of a series of XH molecules towards heterolytic dissociative chemisorption are reviewed, and shown to correlate with their acidities. With ammonia, where non-dissociative adsorption can accompany heterolytic chemisorption, the surface anions of the alkaline earth oxides exhibit strong UV charge-transfer absorption. Analogy is drawn with the behaviour of ammonia in developing charge-transfer-to-solvent spectra with anions in solution. Finally, the propensity of the alkaline earth oxides to produce anions from adsorbed molecules is treated further, and special reference is made to pyridine and to carbon monoxide, where UV-visible spectra show that adsorbed anions couple to give more complex resonance-stabilized structures." @default.
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- W2020737476 date "1985-09-01" @default.
- W2020737476 modified "2023-10-12" @default.
- W2020737476 title "Surface properties of alkaline earth oxides as studied by UV-visible diffuse reflectance spectroscopy" @default.
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- W2020737476 doi "https://doi.org/10.1016/0254-0584(85)90063-x" @default.
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