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- W2020950196 abstract "Abstract From a solution of a Schrodinger-type wave equation with a nonradiative boundary condition based on Maxwell's equations, Mills predicts that atomic hydrogen may undergo a catalytic reaction with certain gaseous ions such as Ar+ which ionize at integer multiples of the potential energy of atomic hydrogen, 27.2 eV . The reaction involves a nonradiative energy transfer to form a hydrogen atom that is lower in energy than unreacted atomic hydrogen with the release of energy. Upon the addition of 5% argon catalyst to a hydrogen plasma, the Lyman α emission was observed to increase by about an order of magnitude which indicated an increase in the plasma temperature; whereas, xenon control had no effect. Thus, the energy balances of argon–hydrogen glow discharge plasmas were measured using Calvet calorimetry. The steady state Calvet voltage significantly increased upon the addition of 3% hydrogen to an argon plasma, and the output signal was integrated until the signal returned to baseline. An energy balance of over −151,000 kJ / mol H2 was measured compared to the enthalpy of combustion of hydrogen of −241.8 kJ / mol H2. Whereas, under identical conditions no change in the Calvet voltage was observed when hydrogen was added to a plasma of xenon which does not provide a reaction with a net enthalpy of a multiple of the potential energy of atomic hydrogen under these conditions." @default.
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- W2020950196 date "2002-09-01" @default.
- W2020950196 modified "2023-09-27" @default.
- W2020950196 title "Measurement of energy balances of noble gas–hydrogen discharge plasmas using Calvet calorimetry" @default.
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