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• W2020990400 abstract "We present an in situ X-ray scattering study of chloride and bromide adsorption onto the Pt(111) surface and the influence of these anions on the underpotential deposition (UPD) of copper. With bromide in solution, we observe an in-plane diffraction pattern that is consistent with a hexagonal, close-packed, bromide monolayer. The monolayer is incommensurate, but aligned with the underlying platinum lattice, and is present over a wide potential range. The in-plane diffraction measurements are correlated with X-ray specular reflectivity results, to confirm the surface coverages and give information about the surface normal structure. The initial adsorption of copper in the presence of bromide or chloride anions also results in an ordered structure with an incommensurate hexagonal unit cell. Changes in the in-plane scattering intensities at X-ray energies close to the Cu K-edge indicate that the adsorbed layer must include both copper and the halide. The data are described by a bilayer structure very similar to the (111) planes of CuCl (or CuBr)." @default.
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• W2020990400 date "1996-04-01" @default.
• W2020990400 modified "2023-10-10" @default.
• W2020990400 title "In situ X-ray scattering study of the Pt(111)-solution interface: Ordered anion structures and their influence on copper underpotential deposition" @default.
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• W2020990400 doi "https://doi.org/10.1016/0921-4526(95)00933-7" @default.
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