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- W2021055566 abstract "The OH2− defect in CaO has been studied by EPR. The 77 K static spectrum has been reinterpreted and new values are given for the spin-Hamiltonian parameters and principal axes orientation. The averaging features due to the motion of the defect at higher temperatures are studied by means of the stochastic Liouville formalism. Inclusion of pseudosecular Hamiltonian terms within the theory explains most of the experimental details. The hopping process follows the classical exponential temperature dependence, with an activation energy of 0.23±0.01 eV. A superhyperfine (shf) structure resolved at room temperature permits identification of a nearest-neighbor substitutional Mg2+ ion as the perturbation that stabilizes the defect. The 25Mg shf and quadrupolar parameters, including their absolute signs, are also given." @default.
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- W2021055566 date "1986-10-15" @default.
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- W2021055566 title "A new EPR study of the OH<sup>2</sup><sup>−</sup> molecular ion in CaO" @default.
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- W2021055566 doi "https://doi.org/10.1063/1.451797" @default.
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