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• W2021244703 abstract "The absorption spectrum of H2O in Ne, Ar, Kr, Xe and ice matrices in the region of the first à 1B1 continuum is reported. Substantial blue gas-to-matrix shifts are observed for the maximum, which increase with decreasing matrix cage size. The absorption thresholds show much weaker shifts. These features are interpreted in terms of Rydbergization of the (3s/4a1) molecular orbital correlated to the à state. The photochemistry is strongly affected by the environmental effects on the excited state potential surface. An energy threshold to photodissociation is confirmed, consistent with a potential barrier due to the cage and a prompt exit of the H fragment. The photodissociation quantum yield shows a linear dependence with excess kinetic energy in Ar and Xe matrices, in agreement with recent MD simulations also favouring prompt exits as the dominant mechanism to permanent dissociation." @default.
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• W2021244703 date "1994-09-01" @default.
• W2021244703 modified "2023-09-24" @default.
• W2021244703 title "Absorption by dissociative continua in condensed matter: H2O in rare gas and ice matrices" @default.
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• W2021244703 doi "https://doi.org/10.1016/0301-0104(94)00166-9" @default.
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