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• W2021447758 abstract "Vibrationally mediated photodissociation combined with Doppler spectroscopy and time-of-flight detection of H-atoms provides information on the photofragmentation dynamics from selected rovibrational states of Ã1A2‘ ‘-state ammonia. The competition between adiabatic dissociation forming excited-state NH2(2A1) + H and nonadiabatic dissociation leading to ground-state NH2(2B1) + H products changes drastically for dissociation from different parent levels prepared by double-resonance excitation. The H-atom speed distributions suggest that the nonadiabatic dissociation channel is the major pathway except for dissociation from the antisymmetric N−H stretching (31) parent level, which forms exclusively NH2(2A1) + H. The energy disposal depends strongly on the parent state with as little as 2% of the available energy channeled into translational energy for dissociation from the 31 state." @default.
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• W2021447758 date "2003-04-26" @default.
• W2021447758 modified "2023-10-05" @default.
• W2021447758 title "Competition between Adiabatic and Nonadiabatic Pathways in the Photodissociation of Vibrationally Excited Ammonia" @default.
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• W2021447758 doi "https://doi.org/10.1021/jp027396g" @default.
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