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• W2021499158 abstract "The effects of self-assembled monolayer templates terminated with carboxyl, hydroxyl, amino and methyl groups (–COOH, –OH, –NH2 and –CH3) on CaCO3 crystallization are compared in aqueous solutions of low, medium and high Ca2+ concentrations. On the –COOH surface, only calcite rhombohedra are crystallized in the solutions at three different concentrations, while size, shape and orientation of the formed calcites are distinct in various Ca2+ concentration solutions. In low Ca2+ concentration solution, vaterites (111) and (200) are formed on –OH and –NH2 surfaces respectively while no crystals are observed on –CH3 surface. In high Ca2+ concentration solution, calcite (104) is formed on the –OH surface. Calcites and small amounts of vaterites and aragonites are formed on –NH2 and –CH3 surfaces. In medium concentration solutions, the results are similar to the case of high concentration with a lower density of crystals. From the view of the two well-known mechanisms for biomineralization, ion absorption and particle-based crystallization, the results in our study are discussed. Our findings can advance the understanding of CaCO3 biomineralization in nature and also supply guidance for the design of advanced biomaterials." @default.
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• W2021499158 date "2012-01-01" @default.
• W2021499158 modified "2023-10-18" @default.
• W2021499158 title "Combined effect of ion concentration and functional groups on surface chemistry modulated CaCO3 crystallization" @default.
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• W2021499158 doi "https://doi.org/10.1039/c2ce25731a" @default.
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