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- W2021525653 abstract "Abstract— To clarify their similarities and common assumptions, a unified derivation is presented of the methods of evaluating the radiative lifetime of an electronically-excited state by integration of the absorption spectrum or of the fluorescence spectrum. Previous examinations of the accuracy of these methods are briefly reviewed. The radiative lifetime of eleven aromatic molecules is computed by the fluorescence spectrum method, and compared with published lifetimes determined experimentally and by integration of the absorption spectrum; from this it is concluded that the fluorescence spectrum method is accurate to about 25 per cent, and that the common assumption of equal partition functions for the ground and excited states is often not true. Extension of the derivation of formulas for the radiative lifetime shows that the standard chemical potential of the excited state may be determined from the experimental radiative lifetime and appropriately scaled integration of the fluorescence spectrum." @default.
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- W2021525653 date "1975-06-01" @default.
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- W2021525653 title "RADIATIVE LIFETIME AND THERMODYNAMIC POTENTIAL OF EXCITED STATES" @default.
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