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- W2021683256 abstract "We present a vibrational study of the $mathrm{CN}/mathrm{Pt}(111)$ system immersed in acetonitrile, using optical sum-frequency generation. Frequencies of $2073mathrm{cm}{}^{ensuremath{-}1}$ (on-top) and $1861mathrm{cm}{}^{ensuremath{-}1}$ (hollow), distinctly above and below that of the isolated molecule, demonstrate a covalent CN-metal bond. Cluster calculations show that the strengthening and weakening of the C-N bond at the on-top and hollow sites is due to a surface-induced depletion of the antibonding $4ensuremath{sigma}$ and bonding $1ensuremath{pi}$ orbitals, respectively. We illustrate our results with a comparison to the reference $mathrm{CO}/mathrm{Pt}(111)$ system." @default.
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- W2021683256 date "1998-01-26" @default.
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- W2021683256 title "Covalent Bonding of CN to the Pt(111) Surface" @default.
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- W2021683256 doi "https://doi.org/10.1103/physrevlett.80.766" @default.
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