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• W2021716322 abstract "B-site substituted ordered double perovskite-type structure BaCa0.33Nb0.67−xFexO3−δ (x = 0.00, 0.17, 0.25, 0.50) (BCNF) was synthesized by conventional solid state method at 1400°C in air. In-situ high temperature powder X-ray diffraction (HT-PXRD) under CO2 displayed a single-phase double perovskite-type structure at 25–800°C, suggesting excellent chemical stability. Selected area electron diffraction (SAED) further supported the PXRD. Physical (e.g., density) and electrical properties (e.g., conductivity, sensitivity) were correlated with amount of Fe content in BCNF. BCNF changed its impedance under CO2 (ppm level) mixed with dry synthetic air (21% CO2 in N2) at 500°C and 700°C. BCNF with the highest Fe-doped, BaCa0.33Nb0.17Fe0.50O3−δ (BCNF50), exhibited an excellent sensitivity (t90 ∼7 min at 500°C and t90 ∼4 min at 700°C) comparing to lower Fe-content BCNF samples. The sensor response (current density) as a function of log CO2 showed a linear behavior. The critical role of Fe in mixed conducting BCNF has been investigated to illustrate its potential applications for real time detection of CO2 in ppm level." @default.
• W2021716322 created "2016-06-24" @default.
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• W2021716322 date "2013-01-01" @default.
• W2021716322 modified "2023-09-25" @default.
• W2021716322 title "Preparation, Structure and CO₂Sensor Studies of BaCa_0.33Nb_0.67−xFe_xO_3−δ" @default.
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• W2021716322 doi "https://doi.org/10.1149/2.043308jes" @default.
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