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- W2021719145 abstract "An investigation of the ultraviolet absorption spectra of $mathrm{K}{mathrm{Z}n}_{1ensuremath{-}xensuremath{-}y}{mathrm{Mn}}_{x}{mathrm{Ni}}_{y}{mathrm{F}}_{3}$ and $mathrm{K}{mathrm{Mn}}_{x}{mathrm{Ni}}_{1ensuremath{-}x}{mathrm{F}}_{3}$ crystals is reported. Two regions of absorption have been found, one near 40 000 ${mathrm{cm}}^{ensuremath{-}1}$ and the other near 45 000 ${mathrm{cm}}^{ensuremath{-}1}$, corresponding to the simultaneous electronic excitation of the ${mathrm{Mn}}^{2+}$ to the $^{4}A_{1g}$, $^{4}{E}_{g}^{a}$ states and the ${mathrm{Ni}}^{2+}$ to its $^{1}E_{g}$ state in the first case, and of ${mathrm{Mn}}^{2+}$ to its $^{4}{E}_{g}^{b}$ state and ${mathrm{Ni}}^{2+}$ to its $^{1}E_{g}$ state in the second. It is shown from a study of the temperature dependence of the intensity that the mechanism for the absorption of light involves exchange-coupled pairs with the selection rule $ensuremath{Delta}S=0$. The oscillator strengths of the lines and the temperature-dependent shifts of the absorption peaks in the spectra of the concentrated crystals can be accounted for using the theoretical model proposed earlier." @default.
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- W2021719145 date "1967-09-10" @default.
- W2021719145 modified "2023-09-27" @default.
- W2021719145 title "Simultaneous Electronic Excitation of Exchange-Coupled Pairs of Manganese and Nickel Ions" @default.
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- W2021719145 doi "https://doi.org/10.1103/physrev.161.207" @default.
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