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- W2021824897 abstract "The 14N nuclear pure quadrupole resonance has been observed in solid S4N4. The spectrum consists of 12 lines assigned to the resonance of nitrogen atoms located at four inequivalent crystallographic sites. The measured quadrupole coupling constants are discussed in terms of the electronic populations of the valence orbitals on the nitrogen atoms. As compared, on a simple sp2 hybridization model, to standard pyridinic compounds, π type orbitals appear to be much more populated in S4N4. It is also shown that the temperature dependence of the ν+ line frequencies is caused by both lattice and intramolecular motions; the deduced frequencies are consistent with the results of ir and Raman spectra." @default.
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- W2021824897 date "1973-11-15" @default.
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- W2021824897 title "14N Nuclear quadrupole resonance in tetrasulfur tetranitride" @default.
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- W2021824897 doi "https://doi.org/10.1063/1.1679885" @default.
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