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• W2022031221 abstract "We predict the existence of a class of ultracold giant molecules formed from trapped ultracold Rydberg atoms and polar molecules. The interaction which leads to the formation of such molecules is the anisotropic charge-dipole interaction ($a/R^2$). We show that prominent candidate molecules such as KRb and deuterated hydroxyl (OD) should bind to Rydberg rubidium atoms, with energies $E_bsimeq 5-25$ GHz at distances $Rsimeq 0.1-1 mu$m. These molecules form in double wells, mimicking chiral molecules, with each well containing a particular dipole orientation. We prepare a set of correlated dressed electron-dipole eigenstates which are used in a resonant Raman scheme to coherently control the dipole orientation and to create cat-like entangled states of the polar molecule." @default.
• W2022031221 created "2016-06-24" @default.
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• W2022031221 date "2010-06-15" @default.
• W2022031221 modified "2023-09-26" @default.
• W2022031221 title "Ultracold Giant Polyatomic Rydberg Molecules: Coherent Control of Molecular Orientation" @default.
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• W2022031221 doi "https://doi.org/10.1103/physrevlett.104.243002" @default.
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