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- W2022046695 abstract "The piston-displacement technique previously described has been applied to a study of phase transitions and isothermal compressibilities of solid CH4, CD4 and O2 over the pressure range 0–19,000 kgcm2 and the temperature range 4–120°K. Phase transitions appear as discontinuities in V (first order) or in (dVdP)T (second order). Solid CH4 and CD4 both show three phases and one triple point. The transitions appear to be of the second order, with rather large “regions of indifference”. There are isotopic differences between the two methanes. At atmospheric pressure CH4 shows only one of the transitions, at 20.5°K, while CD4 has both, at 22.1° and 27.2°K. There is at present disagreement between our results for CH4 and those obtained by Stevenson. In the case of solid oxygen, the two well-known transitions have been traced to high pressure. The lower transition is evidently of the second order. The upper first-order transition has a large volume discontinuity. Some difficulty was experienced from ignition of the steel pressure chambers by the solid oxygen under high pressure. Pressure-volume relations for the three substances have been obtained at various temperatures." @default.
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- W2022046695 date "1960-01-01" @default.
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- W2022046695 title "Phase transitions and compressions of solid CH4, CD4 and O2" @default.
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- W2022046695 doi "https://doi.org/10.1016/0022-3697(60)90029-9" @default.
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