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- W2022052823 abstract "Radical merry-go-round! Diaryl thiocarbonates, available in a single step from phenols, can be directly transformed into benzoates by a new radical cascade that transposes O and C atoms at the aromatic core. The cascade bypasses the common Barton–McCombie fragmentation in favor of the usually unfavorable O-neophyl rearrangement, which is rendered irreversible and efficient by a highly exothermic CS bond scission in the O-centered radical (see scheme; FG=functional group). Detailed facts of importance to specialist readers are published as ”Supporting Information”. Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article." @default.
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- W2022052823 date "2010-07-05" @default.
- W2022052823 modified "2023-10-18" @default.
- W2022052823 title "Radical 1,2-O→C Transposition for Conversion of Phenols into Benzoates by O-Neophyl Rearrangement/Fragmentation Cascade" @default.
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- W2022052823 doi "https://doi.org/10.1002/chem.201001056" @default.
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