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- W2022066566 abstract "By means of a Heitler-London procedure, theoretical expressions for the ESR parameters of a pair of identical complex ions with spin S =(1/2) are derived. The conditions for spin coupling and for a disalignment of the g and fine-structure tensors are discussed. The calculation of the contributions of the dipolar and exchange interactions, respectively, shows that the last one, which causes the singlet-triplet energy separation, gives anisotropic contributions to the zero-field splitting, owing to the effect of the spin-orbit coupling. Moreover, such contributions are in competition with those of the dipolar interaction. The crucial importance, for the exchange interaction, of a mixed ground state is shown. Its dependence on the form of the ligand orbitals is also pointed out." @default.
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- W2022066566 date "1974-11-01" @default.
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- W2022066566 title "Spin coupling of two identical complex ions. I. Theory" @default.
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