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• W2022080493 endingPage "9824" @default.
• W2022080493 startingPage "9819" @default.
• W2022080493 abstract "Over the past several decades, the increased use of artificial sweeteners as dietary supplements has resulted in rising concentrations of these contaminants being detected in influent waters entering treatment facilities. As conventional treatments may not quantitatively remove these sweeteners, radical-based advanced oxidation and reduction (AO/RP) treatments could be a viable alternative. In this study, we have established the reaction kinetics for both hydroxyl (•OH) and sulfate (SO4•–) radical reaction with five common artificial sweeteners, as well as their associated reaction efficiencies. Rate constants for acesulfame K, aspartame, rebaudioside A, saccharin, and sucralose were <2 × 107, (2.28 ± 0.02) × 109, (2.1 ± 0.1) × 108, <2 × 107, and (1.7 ± 0.1) × 108 M–1 s–1 for the sulfate radical, and (3.80 ± 0.27) × 109, (6.06 ± 0.05) × 109, (9.97 ± 0.12) × 109, (1.85 ± 0.01) × 109, and (1.50 ± 0.01) × 109 M–1 s–1 for the hydroxyl radical, respectively. These latter values have to be combined with their corresponding reaction efficiencies of 67.9 ± 0.9, 52.2 ± 0.7, 43.0 ± 2.5, 52.7 ± 2.9, and 98.3 ± 3.5% to give effective rate constants for the hydroxyl radical reaction that can be used in the modeling of the AOP based removal of these contaminants." @default.
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• W2022080493 date "2012-10-01" @default.
• W2022080493 modified "2023-10-17" @default.
• W2022080493 title "Reaction Kinetics and Efficiencies for the Hydroxyl and Sulfate Radical Based Oxidation of Artificial Sweeteners in Water" @default.
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• W2022080493 doi "https://doi.org/10.1021/jp3047246" @default.
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