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- W2022082658 abstract "A series of transition metal substituted polyoxometalates (POMs) have been attached to carbon electrodes in multilayer films of poly(allylamine hydrochloride) (PAH). These include Wells–Dawson-derived sandwich-type Fe4III(H2O)2(As2W15O56)212-, Co4II(H2O)2(As2W15O56)216- and Mn4II(H2O)2(As2W15O56)216- and Wells–Dawson mono-substituted-type α1-[P2W17VIVO62]8− and α2-[P2W17O61(OH)2FeIII]7−. The modified electrodes were characterized by cyclic voltammetry and UV–Vis spectroscopy. The experimental observations indicate the degradation of the substituted-POMs during their incorporation in the PAH multilayer film, probably as a result of electrostatic repulsions between the positively-charged metal cation substitute (FeIII, MnII or VIV) of the POM and the positively-charged PAH. The degradation mostly results in the formation of lacunary-type POMs. Although the encapsulation does not lead to the entire preservation of the substituted-POMs, the substituted-POMs/PAH films can be used as pH sensors and as efficient electrocatalysts for the reduction of dioxygen, hydrogen peroxide and the oxidation of the NADH coenzyme." @default.
- W2022082658 created "2016-06-24" @default.
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- W2022082658 date "2010-07-01" @default.
- W2022082658 modified "2023-10-18" @default.
- W2022082658 title "Attempts to immobilize catalytically active substituted-heteropolytungstates in multilayer film of charged polyelectrolyte poly(allylamine hydrochloride)" @default.
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- W2022082658 doi "https://doi.org/10.1016/j.jelechem.2010.03.026" @default.
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