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- W2022083472 abstract "Abstract The decomposition of dimethyl ether (CH 3 OCH 3 ) has been investigated behind incident shock waves in a diaphragmless shock tube using laser schlieren densitometry, LS ( T = 1500–2450 K, P = 57 ± 4, 125 ± 5 and 253 ± 12 Torr). The LS density gradient profiles were simulated and excellent agreement was found between the simulations and experimental profiles. Rate coefficients for CH 3 OCH 3 → CH 3 O + CH 3 were obtained. They showed strong fall-off, and at the lower end of the experimental temperature range are close to the low pressure limit. First order rate coefficient expressions were determined over 1500 T k 57Torr = (3.10 ± 1.0) × 10 79 T −19.03 exp(−54417/ T ) s −1 , k 125Torr = (1.12 ± 0.3) × 10 83 T −19.94 exp(−55554/ T ) s −1 and k 253Torr = (1.02 ± 0.3) × 10 73 T −17.09 exp(−51500/ T ) s −1 . The effect of a roaming channel for decomposition of dimethyl ether was assessed and the best agreement was obtained with 1% dissociation of DME via the roaming path." @default.
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- W2022083472 date "2013-01-01" @default.
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- W2022083472 title "Dissociation of dimethyl ether at high temperatures" @default.
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- W2022083472 doi "https://doi.org/10.1016/j.proci.2012.05.021" @default.
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