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- W2022088093 abstract "Electrochemistry at DNA-modified surfaces provides an alternative approach to photochemistry or radiation biology for studying charge migration through the double helix. Using short duplexes self-assembled onto gold, electrochemical reduction of redox-active reporter molecules has been observed through DNA films more than 50 A thick, with heterogeneous rate constants as great as approximately 100 s(-1). Though apparently insensitive to base content and sequence, even small distortions in the electronic structure of the pi-stack (caused, for example, by single-base mismatches and other DNA lesions) attenuate the rate of electron transport. Understanding the role of conformational dynamics within the double helix, as well as the cooperative effects of self-assembling individual duplexes into ordered superlattices remain important challenges for theory and experiment." @default.
- W2022088093 created "2016-06-24" @default.
- W2022088093 creator A5017520037 @default.
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- W2022088093 date "2001-04-01" @default.
- W2022088093 modified "2023-09-25" @default.
- W2022088093 title "Electrochemistry at DNA-modified surfaces: new probes for charge transport through the double helix" @default.
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- W2022088093 doi "https://doi.org/10.1016/s1367-5931(00)00192-7" @default.
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