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- W2022101006 abstract "The effect of the water matrix components of a secondary effluent of a urban wastewater treatment plant on the photocatalytic activity of Ag/AgCl @ chiral TiO2 nanofibers and the undergoing reaction mechanisms were investigated. These effects were evaluated through the water components-induced changes on the net rate of hydroxyl radical (OH) generation and modeled using a relative rate technique. Dissolved organic matter DOM (k = −2.8 × 108 M−1 s−1) scavenged reactive oxygen species, Cl− (k = −5.3 × 108 M−1 s−1) accelerated the transformation from Ag to AgCl (which is not photocatalytically active under visible-light irradiation), while Ca2+ at concentrations higher than 50 mM (k = −1.3 × 109 M−1 s−1) induced aggregation of Ag/AgCl and thus all of them revealed inhibitory effects. In contrast, NO3− (k = 6.9 × 108 M−1 s−1) and CO32− (k = 3.7 × 108 M−1 s−1) improved the photocatalytic activity of Ag/AgCl slightly by improving the rate of HO generation. Other ubiquitous secondary effluent components including SO42− (k = 3.9 × 105 M−1 s−1), NH3+ (k = 3.5 × 105 M−1 s−1) and Na+ (k = 2.6 × 104 M−1 s−1) had negligible effects. 90% of 17-α-ethynylestradiol (EE2) spiked in the secondary effluent was removed within 12 min, while the structure and size of Ag/AgCl @ chiral TiO2 nanofibers remained stable. This work may be helpful not only to uncover the photocatalytic mechanism of Ag/AgCl based photocatalyst but also to elucidate the transformation and transportation of Ag and AgCl in natural water." @default.
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- W2022101006 date "2015-03-01" @default.
- W2022101006 modified "2023-10-13" @default.
- W2022101006 title "Mechanism and experimental study on the photocatalytic performance of Ag/AgCl @ chiral TiO2 nanofibers photocatalyst: The impact of wastewater components" @default.
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- W2022101006 doi "https://doi.org/10.1016/j.jhazmat.2014.10.060" @default.
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