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- W2022114282 abstract "The gas-phase laser-induced fluorescence (LIF) spectrum of a 1-phenylpropargyl radical has been identified in the region 20800−22000 cm-1 in a free jet. The radical was produced from discharges of hydrocarbons including benzene. Disregarding C2, C3, and CH, this radical appears as the most strongly fluorescing product in a visible wavelength two-dimensional fluorescence excitation−emission spectrum of a jet-cooled benzene discharge. The structure of the carrier was elucidated by measurement of a matching resonant two-color two-photon ionization spectrum at m/z = 115 and density functional theory. The assignment was proven conclusively by observation of the same excitation spectrum from a low-current discharge of 3-phenyl-1-propyne. The apparent great abundance of the 1-phenylpropargyl radical in discharges of benzene and, more importantly, 1-hexyne may further underpin the proposed importance of the propargyl radical in the formation of complex hydrocarbons in combustion and circumstellar environments." @default.
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- W2022114282 date "2008-02-15" @default.
- W2022114282 modified "2023-09-23" @default.
- W2022114282 title "Spectroscopic Observation of the Resonance-Stabilized 1-Phenylpropargyl Radical" @default.
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- W2022114282 doi "https://doi.org/10.1021/ja078342t" @default.
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