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• W2022121541 endingPage "2203" @default.
• W2022121541 startingPage "2191" @default.
• W2022121541 abstract "A tunable, single frequency, continuous wave, dye laser has been used to optically pump various lines of the BaO A 1Σ-X 1Σ electronic transition. Microwave optical double resonance (MODR) spectra are recorded as changes in the intensity of dye laser induced photoluminescence. Fourteen microwave rotational transitions in the X 1Σ (ν = 0,1) and A 1Σ (ν = 0–5) states of 138Ba16O and one transition in the A 1Σ (ν = 1) state of 137Ba16O have been observed. Partially deperturbed rotational constants obtained for BaO A 1Σ are B(ν) = 0.25832(2) − 0.001070(5) (ν + 1/2) cm−1. Two physical models are described which account for microwave optical double resonance effects in the strong (nonlinear) and weak (linear) optical pumping limits. Observed changes in photoluminescence polarization caused by excited state microwave transitions are predicted by a semiclassical transition dipole model. A three level steady state kinetic treatment of microwave optical double resonance indicates that the BaO MODR transitions reported in this paper are observed near the strong optical pumping limit. It is shown that for most allowed transitions in diatomic molecules a 100 mW single frequency, dye laser is sufficiently intense to significantly deplete rotational levels of the electronic ground state with respect to neighboring rotational levels and to cause the populations of the depleted ground state and optically pumped excited state levels to become comparable." @default.
• W2022121541 created "2016-06-24" @default.
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• W2022121541 date "1973-09-01" @default.
• W2022121541 modified "2023-10-18" @default.
• W2022121541 title "Microwave optical double resonance spectroscopy with a cw dye laser: BaO <i>X</i>1Σ and <i>A</i>1Σ" @default.
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• W2022121541 doi "https://doi.org/10.1063/1.1680320" @default.
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