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• W2022139026 abstract "The adsorption of EDTA on magnetite has been measured as a function of pH and EDTA concentration. The number of anchorage sites of EDTA on magnetite changes from 2 to 4 with increasing pH, while the affinity goes through a maximum in the pH interval 3–4. Adsorption of Fe(II) on EDTA has also been measured, the behavior being similar to that of other hydrolizable ions. The more complex composite systems EDTAFe(II), Fe(III)Fe3O4 are also analyzed and it is concluded that surface and dissolved iron ions compete for EDTA; thus the adsorptivity of the complex ions is less than the adsorptivity of either EDTA or aqueous iron ions. The rates of dissolution of magnetite in EDTA solutions with and without added Fe(II) have been measured and the results interpreted through a much faster rate of phase transfer for Fe(II) as compared to Fe(III). Heterogeneous electron transfer is involved in the dissolution of magnetite by ferrous ions, either exogenous or autogenerated. EDTA is necessary for the reductive pathway, as the larger stability constant of the Fe(III) complex over the Fe(II) complex provides the driving force for the heterogeneous electron transfer." @default.
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• W2022139026 date "1984-04-01" @default.
• W2022139026 modified "2023-10-12" @default.
• W2022139026 title "Adsorption of EDTA and iron—EDTA complexes on magnetite and the mechanism of dissolution of magnetite by EDTA" @default.
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• W2022139026 doi "https://doi.org/10.1016/0021-9797(84)90155-3" @default.
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