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• W2022146313 abstract "The published results of Grimes and Morris on the rate of the uranium-water vapour reaction which were obtained using interferometry have been recalculated using the best values derived from the literature for the complex refractive indices of uranium and uranium dioxide (3.1–3.91 for uranium and 2.2-0.51 for uranium dioxide). The kinetics have been described by Haycock's model and the linear rate constant is given by K 1 = 1.3 × 10 4 P 1 2 H 2 O exp( − 9.0 kcal/RT )mg U/cm 2 h, where P H 2 O is the water vapour pressure in torr or K 1 = 3.48 × 10 8 r 1 2 exp( −14.1 kcal/RT)mg U/cm 2 h, where r is the fractional relative humidity, R is the gas constant and T is the absolute temperature. A mechanism is described which accounts for the observed dependence of the rate of uranium-water vapour reaction on the square root of the water vapour pressure." @default.
• W2022146313 created "2016-06-24" @default.
• W2022146313 creator A5041528668 @default.
• W2022146313 date "1984-04-01" @default.
• W2022146313 modified "2023-09-26" @default.
• W2022146313 title "The kinetics and mechanism of the uranium-water vapour reaction — an evaluation of some published work" @default.
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• W2022146313 doi "https://doi.org/10.1016/0022-3115(84)90052-7" @default.
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