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• W2022207945 endingPage "78" @default.
• W2022207945 startingPage "74" @default.
• W2022207945 abstract "A precipitate was found at the interface between the aqueous phase and the ionic liquid (IL) phase during the separation of U O 2 2 + /Eu 3+ using irradiated IL 1-butyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imides (C 4 mimNTf 2 ), and was analyzed by SEM, EDS, XPS and PXRD. The anions F − and S O 4 2 − were identified as the radiolytic products of C 4 mimNTf 2 . The radiation effect on the extraction of U O 2 2 + from aqueous solution by tri-n-butyl phosphate (TBP) in C 4 mimNTf 2 was studied. For the presence of F − and S O 4 2 − , the utilization of irradiated C 4 mimNTf 2 as diluent reduced the extraction efficiency of U O 2 2 + . The EXAFS measurement showed that the degradation of C 4 mimNTf 2 insignificantly influenced the coordination environment of U O 2 2 + in the IL phase. Furthermore, it was suggested that the complex of uranyl ion with four TBP molecules is predominant during the extraction of U O 2 2 + by TBP in C 4 mimNTf 2 from aqueous solution in the absence of nitric acid. This work gives a further assessment for the application of ILs in the processing of spent nuclear fuel. ► The anions F − and S O 4 2 − were identified as the radiolytic products of C 4 mimNTf 2 . ► Utilization of irradiated C 4 mimNTf 2 reduced the extraction efficiency of U O 2 2 + . ►Uranyl ion with four TBP molecules is predominant during the extraction." @default.
• W2022207945 created "2016-06-24" @default.
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• W2022207945 date "2013-02-01" @default.
• W2022207945 modified "2023-09-28" @default.
• W2022207945 title "Identification of F− and SO42− as the radiolytic products of the ionic liquid C4mimNTf2 and their effect on the extraction of UO22+" @default.
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• W2022207945 doi "https://doi.org/10.1016/j.radphyschem.2012.10.004" @default.
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