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- W2022234482 abstract "Dispersive relaxations typically found in glassy systems stem from a distribution of response times, spread either heterogeneously of homogeneously within the ensemble of sites. To distinguish between these two possibilities we follow the dynamics of dipole solvation, a technique which provides valuable insight on relaxation in both the liquid and the glassy regime. Employing the dynamic mean spherical approximation (MSA) thory, with ϵ(ω) as an input, we calculate the solvation time evolution in the homogeneous and the heterogeneous limits. Due to the remarkable agreement between the homogeneous MSA and the observed solvation in 2-methyltetrahydrofuran at TG + 3 K=94 K we conclude on the homogeneous nature of dispersion of dipolar relaxations." @default.
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- W2022234482 date "1993-12-01" @default.
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- W2022234482 title "Origin of dispersion in dipolar relaxations of glasses" @default.
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- W2022234482 doi "https://doi.org/10.1016/0009-2614(93)e1251-b" @default.
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