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- W2022293206 abstract "The internal fields at the nuclei of ${mathrm{Ga}}^{3+}$, ${mathrm{Al}}^{3+}$, ${mathrm{V}}^{5+}$, ${mathrm{Sc}}^{3+}$, and ${mathrm{In}}^{3+}$ ions present in some iron garnets have been measured by the spin-echo method. Their values at the octahedral $16a$ and tetrahedral $24d$ sites are in agreement with the superexchange process and with the relative ${mathrm{Fe}}^{3+}$-ion configurations on the two sites. The transferred hyperfine fields at the $a$ sites were composed on an isotropic part and a much smaller anisotropic part. The hyperfine field due to a valence $mathrm{ns}$ electron was calculated by using Goudsmit's formula with some appropriate modifications. The fractions ${f}_{s}$ of the unpaired $mathrm{ns}$ spin of these diamagnetic cations were deduced from these calculated values and the isotropic hyperfine fields. It was shown that this $mathrm{ns}$ polarization is much higher for the $a$ site than for the $d$ site in accord with the covalent character of the ${mathrm{Fe}}^{3+}$ ion at the tetrahedral site. The nuclear-quadrupole splittings at two magnetically inequivalent $a$ sites were measured. The electric field gradients without the antishielding effect were then shown to be approximately the same for $S$-state cations at the $a$ sites" @default.
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- W2022293206 date "1973-10-01" @default.
- W2022293206 modified "2023-09-28" @default.
- W2022293206 title "Supertransferred Hyperfine Fields at the Nuclei of Various Diamagnetic Ions in Yttrium Iron Garnet" @default.
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- W2022293206 doi "https://doi.org/10.1103/physrevb.8.3218" @default.
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