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- W2022305089 abstract "The preparation and crystal structures of the n = 2 Ruddlesden−Popper phases Sr2-xLn1+xMn2O7 (0 ≤ x ≤ 0.5, Ln = La, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Y, and Er) are described. The crystal chemistry and stability of this structure is governed by the size of the lanthanide cation. Partial ordering of the Sr2+ and Ln3+ cations occurs between the two available A cation (A = Ln3+, Sr2+) sites, with the smaller lanthanides preferring the site in the rock-salt layer over that in the perovskite block. This ordering is almost complete for the small lanthanides (Tb−Er), and these ordered compounds can be prepared as single phases. Cation disorder in compounds of the larger lanthanides is accompanied by a subtle separation into two n = 2 Ruddlesden−Popper phases, which is apparent only upon detailed inspection of Rietveld refinements of the X-ray profiles. In these cases, the two-phase model is found to be superior to a single phase model with strain broadening included. For a particular lanthanide, both the ease of synthesis of single phases and the extent of cation ordering depend on the manganese oxidation state." @default.
- W2022305089 created "2016-06-24" @default.
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- W2022305089 date "1997-02-01" @default.
- W2022305089 modified "2023-10-16" @default.
- W2022305089 title "Layered Ruddlesden−Popper Manganese Oxides: Synthesis and Cation Ordering" @default.
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- W2022305089 doi "https://doi.org/10.1021/cm960398r" @default.
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