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- W2022320828 abstract "Abstract Zeolite ZSM-5 of Si/Al ratio from 14 to 100, modified with transition metal ions (Fe 3+ , Mn 2+ , Co 2+ ) introduced by means of ionic exchange, showed catalytic activity for propane oxidation already at 330 °C. The use of air as oxidant resulted mainly in carbon oxides, while application of N 2 O led to high selectivity towards propene. Thermal treatment of modified zeolites was a crucial parameter influencing an oxidative activity of the samples. High activity for propane oxydehydrogenation was found for samples calcined at 900 °C, while the calcination at lower temperature (600 °C) resulted in negligible propane conversion. Presence of MFI structure appeared indispensable for the formation of active transition metal complexes, while Si/Al ratio influenced activity and selectivity of catalysts less significantly." @default.
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- W2022320828 date "2003-04-01" @default.
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- W2022320828 title "Propane oxydehydrogenation over transition metal modified zeolite ZSM-5" @default.
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- W2022320828 doi "https://doi.org/10.1016/s0926-860x(02)00504-5" @default.
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