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- W2022332018 abstract "The rotational, vibrational and translational energy distribution for hydrogen (deuterium) molecules desorbing from a vanadium(1 0 0) + O surface have been determined using resonance enhanced multi-photon ionization time-of-flight spectroscopy. The translational energy has been found to be hyper-thermal for all selected internal states. However, the translational energy Ekin for molecules in v=1 is smaller than for those in the vibrational state v=0. The influence of the rotational states J on the translational energy is more complex: for low J-states Ekin increases with J, whereas for high J-states Ekin decreases with increasing J. We have also measured the population of the individual rotational and vibrational states of the desorbing H2 (D2) molecules: In both cases the first excited vibrational state is overpopulated. The population of the J-states is hyper-thermal for low and high J but sub-thermal for medium J." @default.
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- W2022332018 date "2003-07-01" @default.
- W2022332018 modified "2023-09-23" @default.
- W2022332018 title "Determination of the translational, rotational and vibrational degree of freedom for H2 and D2 desorbing from vanadium(100)+O" @default.
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- W2022332018 doi "https://doi.org/10.1016/s0039-6028(03)00331-5" @default.
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