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• W2022357455 abstract "Time-resolved Fourier-transform spectroscopy and two-color laser-induced grating spectroscopy are two new techniques recently employed in this laboratory. We recorded emission in the near infrared region during laser photolysis of HONO2 with a step-scan Fourier-transform spectrometer and achieved temporal resolution in the microsecond range and spectral resolution of 0.1 cm1. Rotationally resolved emission lines of the (0,0) band of the D 2∑+ →A 2∑ + transition of NO in the region 8900-9300 cnv−1 with irregular relative intensities were observed when an ArF excimer laser was used to photodissociate HONO2. The spectroscopic parameters of both D 2∑+ and A 2∑+ states agree with those previously reported. When a narrow-band ArF laser was used, selective rotational levels of the D state of NO were populated depending on the wavelength of the ArF laser. Our results indicate that absorption of a 193-nm photon by NO(υ″ = 1) is responsible for the observed emission. To test the technique of two-color laser-induced grating spectroscopy, we employed the B 3II0U+-X 1∑g + system of I2. Background-free spectra with transitions involving rotationally selected states were recorded. Various experimental schemes were employed with population gratings formed in either the B or X state. Signals due to different four-wave mixing schemes were distinguished by variation of relative timing between the grating beams and the probe beam." @default.
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• W2022357455 date "1995-04-01" @default.
• W2022357455 modified "2023-09-26" @default.
• W2022357455 title "New Spectral Techniques: Time-Resolved Fourier-Transform Spectroscopy and Two-Color Laser-Induced Grating Spectroscopy" @default.
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• W2022357455 doi "https://doi.org/10.1002/jccs.199500030" @default.
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