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- W2022359844 abstract "The 16-μm bending fundamentals (ν4) of 12CF4, 13CF4, and 14CF4 have been observed at Doppler-limited resolution using a tunable PbSnSe semiconductor diode laser. The tetrahedral splittings of the rotational manifolds have been observed in all three branches, and in particular the dense and partially overlapping transitions in the Q branches have been resolved and assigned. A least-squares fit of the Hamiltonian, including off-diagonal terms, yielded five scalar and three tensor spectroscopic constants for each of the three isotopes. From these constants the upper-state rotational constant B4 and the Coriolis constant ζ4 have been calculated, together with some of the other molecular constants. An absorption feature at about 0.18 cm−1 to the red of the main Q branch of each isotopic species has been identified as the Q branch of (ν2 + ν4) − ν2, which is the transition that lases when CF4 is pumped by a CO2 laser at 9.4 μm (i.e., in ν2 + ν4)." @default.
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- W2022359844 date "1980-10-01" @default.
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- W2022359844 title "High-resolution spectroscopy of the 16-μm bending fundamental of CF4" @default.
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- W2022359844 doi "https://doi.org/10.1016/0022-2852(80)90068-5" @default.
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