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- W2022366534 abstract "Abstract Laser ion-molecule reaction interaction through long range dipole moments leads to potential energy surface crossings. We will show here by using gauge representation (electric field gauge) for wave length λ = 20.6 μm, Intensity I = 5×10 12 W/cm 2 , I = 1×10 13 W/cm 2 , I = 3×10 13 W/cm 2 , that we can create laser induced potential energy surface crossing in the virtual transition state region (4.a.u.) where the dipole moment changes sign. We illustrate such effects for the Li H + CH 3 + ↔ Li + + CH 4 reaction which takes the form of inverted Morse (without a barrier) using ab-initio methods for calculating the reaction path and the permanent dipole moment of this ion-molecule reaction." @default.
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- W2022366534 date "2008-12-01" @default.
- W2022366534 modified "2023-09-25" @default.
- W2022366534 title "Laser Induced Potential Energy Surface Crossing in Ion-Molecule Reactions: Application to Li<sup>+</sup>+CH<sub>4</sub>" @default.
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- W2022366534 doi "https://doi.org/10.1524/zpch.2008.5435" @default.
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