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- W2022368375 abstract "Following exposure to ppm-level hydrogen sulfide at elevated temperatures, a section of a solid oxide fuel cell (SOFC) Ni-YSZ anode was examined using a combination of synchrotron-based x-ray nanotomography and x-ray fluorescence techniques. While fluorescence measurements provided elemental identification and coarse spatial mapping, x-ray nanotomography was used to map the detailed 3-D spatial distribution of Ni, YSZ, and a nickel-sulfur poisoning phase. The nickel-sulfur layer was found to form a scale covering most of the exposed nickel surface, blocking most fuel reformation and hydrogen oxidation reaction sites. Although the exposure conditions precluded the ability to develop a detailed kinetic description of the nickel-sulfur phase formation, the results provide strong evidence of the detrimental effects of 100 ppm hydrogen sulfide on typical Ni-YSZ anode materials." @default.
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- W2022368375 date "2014-06-10" @default.
- W2022368375 modified "2023-10-06" @default.
- W2022368375 title "Three-Dimensional Microstructural Imaging of Sulfur Poisoning-Induced Degradation in a Ni-YSZ Anode of Solid Oxide Fuel Cells" @default.
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- W2022368375 doi "https://doi.org/10.1038/srep05246" @default.
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