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- W2022381864 abstract "An improved version of the recently developed non-Markovian energy corrected sudden (ECS) model [J. V. Buldyreva and L. Bonamy, Phys. Rev. A 60, 370 (1999)] is proposed to ensure good accuracy of the quasiexponential behavior of the scattered light intensity vs frequency that is observed experimentally in the far wings of nitrogen spectra. To this end, the more refined translational spectrum proposed by Birnbaum and Cohen [Can. J. Phys. 54, 593 (1976)] is used as the adiabaticity factor. At low frequencies it reduces to the traditional one-parameter Lorentzian shape which describes the long-time translational dynamics and allows the basic ECS transition rates to be identified. At high frequencies it introduces an additional parameter which describes the short-time dynamics. The value of this parameter at room temperature and at low temperature (150 K) is obtained by fitting the far-wing theoretical intensities of the depolarized nitrogen spectra to their experimental values. This value compares favorably with its theoretical evaluation." @default.
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- W2022381864 date "2000-12-13" @default.
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- W2022381864 title "Non-Markovian far-wing rotational Raman spectrum from translational modeling" @default.
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