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• W2022386515 abstract "The electrical transport properties of hydrohalogenic acid in a Nafion 117 perfluorosulfonic membrane are studied. The conductivity of the membrane material is determined by ac impedance measurements. In membranes previously equilibrated with aqueous solutions, the swelling is modified and the amount of sorbed acid species is evaluated. For higher swelling, the presence of sorbed HF does not affect the membrane conductivity, whereas the presence of HCl and HBr increases it strongly when the fraction of sorbed acid molecules over fixed sulfonic groups is less than 5% for HCl and 20% for HBr. For larger amounts of sorbed HC1 and HBr, the membrane conductivity remains constant. Radiotracer flux measurement of chloride ions shows that the transport number of this anion does not exceed 0.02. These results suggest that the superselectivity of this membrane to protons has two distinct origins: a reduced dissociation of sorbed acid in the membrane phase and an increase of the proton mobility resulting from the sorption of acid." @default.
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• W2022386515 date "1989-02-01" @default.
• W2022386515 modified "2023-10-16" @default.
• W2022386515 title "Conductivity of sorbed hydrohalogenic acid in Nafion perfluorosulfonic membranes" @default.
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• W2022386515 doi "https://doi.org/10.1016/0022-0728(89)80042-7" @default.
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