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• W2022407653 startingPage "2130" @default.
• W2022407653 abstract "A characteristic time scale of order 100 ps has been observed by several workers in picosecond spectroscopy experiments on iodine recombination in liquid CCl4 and other solvents. This time scale has been thought to be associated with the diffusive relative motion, prior to actual recombination, of photodissociated I atoms. In this paper, we point out that extensive vibrational deactivation of nascent iodine molecules formed in the recombination is required for spectroscopic detection of I2. We propose that slow vibrational relaxation of nascent I2 may play an important role in such recombination studies. We examine the relaxation of highly vibrationally excited I2 in liquid CCl4. Both vibrational‐translational (VT) and vibrational–vibrational (VV) energy transfer mechanisms are considered. We estimate that the characteristic time scale for the vibrational relaxation of I2 in CCl4 is of order 100 ps. VV energy transfer is found to play a critical role in the relaxation. Possible experimental avenues for testing our conclusions are suggested." @default.
• W2022407653 created "2016-06-24" @default.
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• W2022407653 date "1982-08-15" @default.
• W2022407653 modified "2023-09-27" @default.
• W2022407653 title "Slow vibrational relaxation in picosecond iodine recombination in liquids" @default.
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• W2022407653 doi "https://doi.org/10.1063/1.444019" @default.
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