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- W2022478342 abstract "In Part II, we extend the inverse methodology which is discussed in Part I to various experiments performed in a tubular reactor to infer mass transfer coefficients. Mass transfer coefficients, inferred from the concentrations of the reactants which are extracted from the absorbance of the reaction mixture using multicomponent spectrum analysis, are then used to solve the convection–diffusion–reaction equations for the concentrations of the reactants in the bulk phase and in the dispersed phase, to explore the possibility of cross-over for a mass transfer limited reaction. Experiments are performed incorporating the asymmetry in the transport rates of the premixed reactants, which is the potential reason for the existence of cross-over. The different mass transfer coefficients of the two premixed reactants indeed indicate a switch in the concentration of the reactants in the dispersed phase, which is termed as “cross-over”. The experimental results are further analysed by validating the theoretical criterion proposed by Mchedlov-Petrossyan et al. (2003, Chem. Eng. Sci. 58, 3005–3023 & 2691–2703) to obtain the parametric space for the existence of cross-over, in order to optimize the length of the tubular reactor." @default.
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- W2022478342 date "2005-08-01" @default.
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- W2022478342 title "Experimental study of mass transfer limited reaction—Part II: Existence of cross-over phenomenon" @default.
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