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- W2022507577 abstract "Dynamic studies of the hydrogenation of α-methyl styrene in a three-phase slurry reactor showed that catalyst reduction temperature appreciably affects individual values of adsorption equilibrium constants, adsorption rate coefficients and surface reaction rate coefficients. Measurements were made in a well-stirred slurry reactor with Pd/Al2O3 catalyst particles at 22, 38 and 50°C. Increasing the temperature for reducing, in hydrogen, PdCl2 to Pd from 250 to 420 to 510°C decreased the palladium dispersion, and caused a reduction in equilibrium adsorption, adsorption rate and surface reaction rate coefficients. The heat of adsorption and the activation energy for surface reaction, 3.8 and 10 kcal/mole, respectively, were constant with reduction temperature. The relative magnitudes of metal dispersion at the three catalyst reduction temperatures were estimated from equilibrium adsorption coefficients, and found to agree with an experimental study by Boitiaux et al. (1983a)." @default.
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- W2022507577 date "1987-01-01" @default.
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- W2022507577 title "Effect of hydrogenation catalyst activity on adsorption and surface reaction rates" @default.
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- W2022507577 doi "https://doi.org/10.1016/0009-2509(87)85059-5" @default.
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