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• W2022615102 endingPage "13734" @default.
• W2022615102 startingPage "13727" @default.
• W2022615102 abstract "Crystalline Si(111) surfaces have been alkylated in a two-step chlorination/alkylation process using various organic molecules having similar backbones but differing in their C-C bond closest to the silicon surface (i.e., C-C vs C=C vs C[triple bond]C bonds). X-ray photoelectron spectroscopic (XPS) data show that functionalization of silicon surfaces with propenyl magnesium bromide (CH3-CH=CH-MgBr) organic molecules gives nearly full coverage of the silicon atop sites, as on methyl- and propynyl-terminated silicon surfaces. Propenyl-terminated silicon surface shows less surface oxidation and is more robust against solvent attacks when compared to methyl- and propynyl-terminated silicon surfaces. We also show a secondary functionalization process of propenyl-terminated silicon surface with 4'-[3-Trifluoromethyl-3H-diazirin-3-yl]-benzoic acid N-hydroxysuccinimide ester [TDBA-OSu] cross-linker. The Si-CH=CH-CH3 surfaces thus offer a means of attaching a variety of chemical moieties to a silicon surface through a short linking group, enabling applications in molecular electronics, energy conversion, catalysis, and sensing." @default.
• W2022615102 created "2016-06-24" @default.
• W2022615102 creator A5037852312 @default.
• W2022615102 creator A5063277241 @default.
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• W2022615102 date "2008-09-20" @default.
• W2022615102 modified "2023-09-23" @default.
• W2022615102 title "Highly Stable Organic Monolayers for Reacting Silicon with Further Functionalities: The Effect of the C−C Bond nearest the Silicon Surface" @default.
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• W2022615102 doi "https://doi.org/10.1021/ja804674z" @default.
• W2022615102 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18803387" @default.
• W2022615102 hasPublicationYear "2008" @default.
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