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- W2022641489 abstract "The collision-induced dissociation (CID) and charge transfer (CT) cross sections for H+2 (υ = O to υ = 10) reactants with H2 have been measured by threshold photoelectron-photoion coincidence (TPEPICO)_at center-of-mass translational energies of 4, 8, 12 and 16 eV. The relative cross sections, normalized by using the known absolute charge transfer cross sections for H+2 (υ = 0 and 1), exhibit a marked dependence on the H+2 vibrational energy. The CID cross sections increase from less than 1 Å2 for υ = 0 to more than 6 Å2 for υ = 10, while the CT cross section decreases from about 11 to 3 Å2. One observes a much weaker variation with translational energy. The analysis of the H+ product ion time of flight distribution shows that the H+ ions are formed in a distribution of kinetic energies which peaks at both low and high laboratory kinetic energies. A direct dissociation model in which the projectile ion is excited to the repulsive 2Σ+u surface is consistent with the observation of fast H+ ions. If the CID is preceded by a charge transfer step, then the same mechanism will give rise to the slow H+ product ions. The ratio of fast to slow H+ ions is unity for low υ but increases as υ increases. This is consistent with the observed decreasing charge transfer cross section with increasing υ." @default.
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- W2022641489 date "1988-01-01" @default.
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- W2022641489 title "The charge transfer and collision-induced dissociation cross sections of state-selected H+2 and D+2 ions" @default.
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- W2022641489 doi "https://doi.org/10.1016/0301-0104(88)80014-4" @default.
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