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• W2022673361 abstract "The further development of Fe0-based remediation technology depends on the profound understanding of the mechanisms involved in the process of aqueous contaminant removal. The view that adsorption and co-precipitation are the fundamental contaminant removal mechanisms is currently facing a harsh scepticism. Results from electrochemical cementation are used to bring new insights in the process of contaminant removal in Fe0/H2O systems. The common feature of hydrometallurgical cementation and metal-based remediation is the heterogeneous nature of the processes which inevitably occurs in the presence of a surface scale. The major difference between both processes is that the surface of remediation metals is covered by layers of own oxide(s) while the surface of the reducing metal in covered by porous layers of the cemented metal. The porous cemented metal is necessarily electronic conductive and favours further dissolution of the reducing metal. For the remediation metal, neither a porous layer nor a conductive layer could be warrant. Therefore, the continuation of the remediation process depends on the long-term porosity of oxide scales on the metal surfaces. These considerations rationalized the superiority of Fe0 as remediation agent compared to thermodynamically more favourable Al0 and Zn0. The validity of the adsorption/co-precipitation concept is corroborated." @default.
• W2022673361 created "2016-06-24" @default.
• W2022673361 creator A5069325712 @default.
• W2022673361 date "2010-09-01" @default.
• W2022673361 modified "2023-10-16" @default.
• W2022673361 title "Elemental metals for environmental remediation: Learning from cementation process" @default.
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• W2022673361 doi "https://doi.org/10.1016/j.jhazmat.2010.05.085" @default.
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