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- W2022674804 abstract "Thin films of uranium oxide, formed by treating cleavage faces of single-crystal UC in purified oxygen, were measured with the help of two optical methods based on ellipsometry. The characteristics of fine-scale oxidation were thus determined at 5 temperatures in the range from 60 °C to 160 °C. In the main, the isothermal growth of the oxide layer appears to be parabolic, with thickness increasing linearly in the square root of the oxidation time; the rate-constant of the process is thermally activated. Both features are indicative of a diffusion-limited process, in which the reaction proceeds by way of oxygen migration through the growing film. In this frame, a qualitative argument indicates that the observed heat of activation can be connected to the migration energy of the oxygen atoms (or ions) in the oxide layer. The estimate for the latter is 25 kcal/mol, in good agreement with the data from diffusion experiments in UO2." @default.
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- W2022674804 date "1968-06-01" @default.
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- W2022674804 title "Growth of oxide films onto cleavage faces of crystalline UC" @default.
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- W2022674804 doi "https://doi.org/10.1016/0039-6028(68)90103-9" @default.
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